| 1 | Charade |
| 2 | MichelleConductor, Arranged By, Producer – George MartinWritten-By – John Lennon/Paul MyCartney |
| 3 | What A Wonderful WorldConductor, Arranged By – Colin KeyesProducer – John BurgessWritten-By – Robert Thiele, George Weiss |
| 4 | No Me Dejes (If You Go Away) |
| 5 | This Is My Life |
| 6 | Fly Me To The Moon (In Other Words) |
| 7 | For All We KnowConductor, Arranged By – Colin KeyesProducer – John BurgessWritten-By – Fred Coots, Samuel Lewis |
| 8 | When I Fall In Love |
| 9 | I Don't Want To Run Your Life |
| 10 | No Puedo Quitar Mis Ojes De Ti (Can't Take My Eyes Off You) |
| 11 | More |
| 12 | Fools Rush In (Where Angels Fear To Tread) |
| 13 | A Lot Of Living |
| 14 | I Have Dreamed |
| 15 | You're Closer To Me |
| 16 | Alguien Canto (The Music Played)Conductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Leonardo Schultz, Udo Jürgens |
| 17 | Hava Nagila |
| 18 | Over The RainbowConductor, Arranged By – Colin KeyesProducer – John BurgessWritten-By – E.Yip Harburg, Harold Arlen |
| 19 | On A Wonderful Day Like TodayConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Anthony Newley, Leslie Bricusse |
| 20 | The Party's Over |
| 21 | Let Me Sing And I'm Happy |
| 22 | Ebb Tide |
| 23 | The Impossible DreamConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Joe Darion, Mitch Leigh |
| 24 | StardustConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Hoagy Carmichael, Mitchell Parish |
| 25 | Listerine / Hartley's Peas / Horniman's Tea |
| 26 | You're SensationalConductor, Arranged By – Colin KeyesProducer – John BurgessWritten-By – Cole Porter |
| 27 | Everybody's Talkin'Conductor, Arranged By – Kenny ClaytonProducer – George MartinWritten-By – Fred Neil |
| 28 | Music To Watch Girls ByConductor, Arranged By – Billy MayProducer – Dave CavanaughWritten-By – Sydney Ramin, Anthony Velona |
| 29 | You're Gonna Hear From MeConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Andre Previn, Dory Previn |
| 30 | On A Clear Day You Can See ForeverConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Alan Ray Lerner, Burton Lane |
| 31 | Love Is A Many Splendored ThingConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Paul Francis Webster, Sammy Fain |
| 32 | September SongConductor, Arranged By – John Cameron Producer – George MartinWritten-By – Kurt Weill, Maxwell Anderson |
| 33 | The Long And Winding Road |
| 34 | Portrait Of My LoveConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Cyril Ornadel, David West |
| 35 | You And Me Against The World |
| 36 | Honey On The Vine |
| 37 | People |
| 38 | Bridge Over Troubled Water |
| 39 | Singin' In The Rain |
| 40 | Softly As I Leave You |
| 41 | When You Wish Upon A Star |
| 42 | Be My Lady |
| 43 | Autumn Leaves |
| 44 | For Once In My LifeConductor, Arranged By – Kenny ClaytonProducer – George MartinWritten-By – Orlando Murden, Ronald Miller |
| 45 | Walk Away |
| 46 | I Get Along Without You Very WellConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Hoagy Carmichael |
| 47 | As Long As She Needs MeConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Lionel Bart |
| 48 | Miss Brown To You |
| 49 | You've Myde Me So Very Happy |
| 50 | Georgia On My MindConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Hoagy Carmichael, Stuart Gorrell |
| 51 | I've Got The Moon On My Side (Unedited) |
| 52 | The Shadow Of Your Smile |
| 53 | Spring Is Here |
| 54 | The Auction |
| 55 | Exodus |
| 56 | SomewhereConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Leonard Bernstein, Stephen Sondheim |
| 57 | Who Can I Turn To |
| 58 | Memory |
| 59 | Gonna Build A MountainConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Anthony Newley, Leslie Bricusse |
| 60 | The Green Leaves Of Summer |
| 61 | You Keep Me Swingin' |
| 62 | Real Life Girl |
| 63 | Zal / The Wonder Of Woolworths / Go Bowling |
| 64 | The Good LifeConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Jack Reardon, Sacha Distel |
| 65 | I Will Wait For YouConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Michel Legrand, Norman Gimbel |
| 66 | Didn't We |
| 67 | You've Got Possibilities |
| 68 | If I Never Sing Another Song |
| 69 | Hey (For Me) |
| 70 | On Days Like These |
| 71 | I Should Care |
| 72 | The Sweetest Sounds |
| 73 | Todo Pasara |
| 74 | Around The World |
| 75 | A Place In Paris |
| 76 | Before You Got |
| 77 | Till The End Of Time |
| 78 | L'etoile Du Sud (The Southern Star) |
| 79 | Sunrise Sunset |
| 80 | I'm Glad There Is YouConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Jimmy Dorsey, Paul Mertz |
| 81 | YesterdayConductor, Arranged By, Producer – George MartinWritten-By – John Lennon/Paul MyCartney |
| 82 | He Ain't Heavy, He's My BrotherConductor, Arranged By – Kenny ClaytonProducer – George MartinWritten-By – Bobby Scott, Sidney Russell |
| 83 | I'm A Fool To Want You |
| 84 | My Way |
| 85 | When Joanna Love MeConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Jack Segal, Robert Wells |
| 86 | Let There Be Love |
| 87 | From Russia With Love |
| 88 | Maria |
| 89 | My Kind Of Girl |
| 90 | The Second Time Around |
| 91 | If She Walked Into My Life |
| 92 | Strangers In The NightConductor, Arranged By – Sid FellerProducer – Dave CavanaughWritten-By – Bert Kaempfert, Charles Singleton, Eddie Snyder |
| 93 | Fourth Blue Monday |
| 94 | Sweet Talkin' Hannah |
| 95 | Born FreeProducer – Ron RichardsWritten-By – Don BlackWritten-By, Conductor, Arranged By – John Barry |
| 96 | Time After TimeConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Jule Styne, Sammy Cahn |
| 97 | My Friend My FriendConductor, Arranged By – Johnnie SpenceProducer – George MartinWritten-By – Domenico Modugno, Hal Shaper |
| 98 | Come Back To Me |
| 99 | We're Gonna Change The World |
| 100 | The Days Of Wine And RosesConductor, Arranged By – Kenny ClaytonProducer – George MartinWritten-By – Henry Mancini, Johnny Mercer |