| 1 | –Robert Goulet | The Girl That I Marry |
| 2 | –Johnny Mathis | Maria From West Side Story |
| 3 | –Percy Faith & His Orchestra | The Way We Were |
| 4 | –Patti Page | Tennessee Waltz |
| 5 | Side H "My Melody Of Love - A World Of Love" |
| 6 | Side A "All The Things You Are - The Great Romantic Themes" |
| 7 | Record 6 |
| 8 | –Andy Williams | We've Only Just Begun |
| 9 | –Andy Williams | Mona Lisa |
| 10 | –Percy Faith & His Orchestra | Stars Fell On Alabama |
| 11 | –Jerry Vale | Al Di La |
| 12 | Side K "Tennessee Waltz - From Country With Love" |
| 13 | –Patti Page | Something |
| 14 | –Vikki Carr | Somos Novios (It's Impossible) |
| 15 | –John Davidson | Happy Heart |
| 16 | Record 7 |
| 17 | Side C "Somewhere, My Love - Hollywood's Great Romantic Hits" |
| 18 | –Percy Faith & His Orchestra | Baubles, Bangles And Beads |
| 19 | –Johnny Mathis | You Are The Sunshine Of My Life |
| 20 | –Patti Page | Can't Help Falling In Love |
| 21 | –Percy Faith & His Orchestra | Easy To Love |
| 22 | Side M "Stardust - Silvery Songs Of Yesteryear" |
| 23 | –Tony Bennett | The Shadow Of Your Smile |
| 24 | –Andy Williams | I Will Wait For You |
| 25 | Side N "Till The End Of Time - Love Songs From The Classics" |
| 26 | –Marty Robbins | Love Me Tender |
| 27 | –Jerry Vale | Arrivederci, Roma |
| 28 | –Andy Williams | Where Or When From Babes In Arms |
| 29 | Side F "Some Enchanted Evening - A Night At The Theater" |
| 30 | –Doris Day | It Had To Be You |
| 31 | –Jerry Vale | Some Enchanted Evening From South Pacific |
| 32 | –Anita Bryant | My Cup Runneth Over From I Do! I Do! |
| 33 | –Andy Williams | Anniversary Song |
| 34 | –The Ray Conniff Singers | Laughter In The Rain |
| 35 | –Vikki Carr | One Less Bell To Answer |
| 36 | –Robert Goulet | The Nearness of You |
| 37 | –Aretha Franklin | Friendly Persuasion |
| 38 | Record 3 |
| 39 | –Andy Williams | Moon River |
| 40 | –Crystal Gayle | Lover Man (Oh, Where Can You Be?) |
| 41 | –André Kostelanetz | Tenderly |
| 42 | Side E "Love Me With All Your Heart - Sweet Sounds Of The '60s" |
| 43 | Record 4 |
| 44 | –Percy Faith & His Orchestra | Theme From A Summer Place |
| 45 | –Johnny Mathis | Stardust |
| 46 | Record 5 |
| 47 | –Mike Douglas | "A"-You're Adorable (The Alphabet Song) |
| 48 | –Jerry Vale | To Each His Own |
| 49 | –Peter Nero | Love Theme From The Godfather |
| 50 | –Jerry Vale | Be My Love |
| 51 | –Jim Nabors | Til The End Of Time |
| 52 | –Tammy Wynette | The Hawaiian Wedding Song |
| 53 | –Tony Bennett | I Left My Heart In San Francisco |
| 54 | –Andy Williams | Love Theme From Romeo And Juliet (A Time For Us) |
| 55 | –Charlie Rich | Behind Closed Doors |
| 56 | –Lynn Anderson | I Love How You Love Me |
| 57 | –The Ray Conniff Singers | My Eyes Adored You |
| 58 | –Johnny Mathis | Feelings |
| 59 | –Norman Luboff Choir | No Other Love |
| 60 | –Vikki Carr | The First Time I Ever Saw Your Face |
| 61 | –Johnny Mathis | Theme From Love Story |
| 62 | –Percy Faith & His Orchestra | Killing Me Softly With Her Song |
| 63 | Side J "Long Ago And Far Away - The Unforgettable '40s" |
| 64 | –Vic Damone | If Ever I Would Leave You From Camelot |
| 65 | –André Kostelanetz | How Deep Is Your Love |
| 66 | –The Ray Conniff Singers | All By Myself |
| 67 | –Doris Day | You'll Never Know |
| 68 | –Doris Day, Robert Goulet | They Say It's Wonderful From Annie Get Your GunConductor – Franz Allers |
| 69 | –Lynn Anderson | Sometimes When We Touch |
| 70 | Side B "My Funny Valentine - Memorable Songs Of The '30s" |
| 71 | Record 2 |
| 72 | –Robert Goulet | What Now My Love |
| 73 | –Tony Bennett, Frank De Vol And His Orchestra | Long Ago (And Far Away) |
| 74 | –Robert Goulet | My Love, Forgive Me (Amore, Scusami) |
| 75 | –Dionne Warwick | Alfie |
| 76 | Side D "Feelings - Beautiful Songs Of Today" |
| 77 | –The Ray Conniff Singers | Somewhere, My Love (Love Theme From Doctor Zhivago) |
| 78 | –Patti Page | Old Cape Cod |
| 79 | –Vikki Carr | For All We Know |
| 80 | –Jerry Vale | Love Is A Many-Splendored Thing |
| 81 | –Percy Faith & His Orchestra | A Lover's Concerto |
| 82 | –Peter Nero | (They Long To Be) Close To You |
| 83 | –Bobby Vinton | This Guy's In Love With You |
| 84 | Side I "You Are The Sunshine Of My Life - Warm And Happy Sounds Of The '70s" |
| 85 | –Engelbert Humperdinck | You Light Up My Life |
| 86 | –Andy Williams | Embraceable You |
| 87 | –Engelbert Humperdinck | Love Me With All Your Heart |
| 88 | –Johnny Mathis | Evergreen (Love Theme From A Star Is Born) |
| 89 | –Andy Williams | Can't Get Use To Losing You |
| 90 | –Vic Damone | You're Breaking My Heart (Mattinata) |
| 91 | Side G "Love Is A Many-Splendored Thing - The Fabulous '50s" |
| 92 | –Tony Bennett | My Funny Valentine |
| 93 | –Johnny Mathis | All The Things You Are |
| 94 | –The Ray Conniff Singers | You Made Me Love You |
| 95 | –The Ray Conniff Singers | My Melody Of Love |
| 96 | –Norman Luboff Choir | Full Moon And Empty Arms |
| 97 | –Norman Luboff Choir | Paper Doll |
| 98 | –Andy Williams | The Song From Moulin Rouge (Where Is Your Heart) |
| 99 | Record 1 |
| 100 | Side L "Arrivederci, Roma - And Other Great Italian Favorites" |
| 101 | –Jerry Vale | Auf Wiederseh'n, Sweetheart |